The actor, who has also appeared in Fear the Walking Dead, will voice the Caped Crusader in The Riddler: Secrets In The Dark.
The Spotify limited series will also include the voices of comedian Hasan Minhaj, who will portray titular villain The Riddler, and Jane the Virgin's Gina Rodriguez as Barbara Gordon.
Also on board are Harry Potter's Jason Isaacs as Alfred, American Vandal's Calum Worthy as The Messenger, New Girl's Hannah Simone as Nadira, and Law & Order: SVU's Peyton Crim as Killer Croc.
Red Dead Redemption 2's Jim Pirri will voice Arnold Flass, Mythic Quest's Ashly Burch will play Vicki Vale, Deadpool's Hugh Scott will portray Calendar Man, The Book of Queer's Bri Giger will voice Summer Gleeson, The Morning Show's Aflamu Johnson is King Tut and 1923's Amy Argyle voices Bat-Tech.
Secrets in the Dark sees Batman team up with The Riddler after a mysterious vigilante starts to kill Gotham's villains, with the series set to premiere on October 10.
The historical drama debuted to an impressive score on Rotten Tomatoes – currently standing at 90% – and is already earning awards buzz for Domingo's performance.
Deadline said that the star "blows through the title role like a force of nature," while TheWrap called his turn an "unforgettable performance".
The Riddler: Secrets In The Dark will debut on Spotify on October 10.
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